Subjects: Optics >> Quantum optics submitted time 2023-02-19
Jing Wang
Nannan Han
Zheng-Dong Luo
Mingwen Zhang
Xiaoqing Chen
Yan Liu
Yue Hao
Jianlin Zhao
Xuetao Gan
Abstract： Electrical tuning of second-order nonlinearity in optical materials is attractive to strengthen and expand the functionalities of nonlinear optical technologies, though its implementation remains elusive. Here, we report the electrically tunable second-order nonlinearity in atomically thin ReS2 flakes benefiting from their distorted 1T crystal structure and interlayer charge transfer. Enabled by the efficient electrostatic control of the few-atomic-layer ReS2, we show that second harmonic generation (SHG) can be induced in odd-number-layered ReS2 flakes which are centrosymmetric and thus without intrinsic SHG. Moreover, the SHG can be precisely modulated by the electric field, reversibly switching from almost zero to an amplitude more than one order of magnitude stronger than that of the monolayer MoS2. For the even-number-layered ReS2 flakes with the intrinsic SHG, the external electric field could be leveraged to enhance the SHG. We further perform the first-principles calculations which suggest that the modification of in-plane second-order hyperpolarizability by the redistributed interlayer-transferring charges in the distorted 1T crystal structure underlies the electrically tunable SHG in ReS2. With its active SHG tunability while using the facile electrostatic control, our work may further expand the nonlinear optoelectronic functions of two-dimensional materials for developing electrically controllable nonlinear optoelectronic devices.
Peer Review Status:
Awaiting Review
Subjects: Optics >> Quantum optics submitted time 2023-02-19
Jing Wang
Peng Yuan
Dongfang Zhang
Guoqiang Xie
Kainan Xiong
Xiaoniu Tu
Yanqing Zheng
Jingui Ma
Liejia Qian
Abstract： Optical quadratic nonlinearity is ultrafast in nature, while parametric interaction usually manifests only the broadband characteristic. Enormous progress has been made toward broadband phase-matching for parametric amplification and wide applications. In existing devices of broadband parametric amplification, the power efficiency of conversion is restricted to approximately the energy efficiency, and the desire for the signal power enhancement necessitates additional pulse compression after amplification. Here, we demonstrate ultrafast parametric amplification having an extraordinary power efficiency of 1155%; this allows the generation of intense femtosecond pulses without the need for a pulse stretcher and compressor. Direct femtosecond signal amplification by picosecond pumping is enabled by an ultrafast parametric environment in which the pre-delayed signal of faster speed gradually overtakes and effectively depletes the pump of slower speed as they propagate in a nonlinear crystal. The demonstrated technique should lead to breakthroughs in ultrafast lasers as well as applications.
Peer Review Status:Awaiting Review
Subjects: Optics >> Quantum optics submitted time 2023-02-19
Abstract： Bio-compatible Au nanoparticles exhibit great advantages in the application of biomedical researches, such as bio-sensing, medical diagnosis, and cancer therapy. Bio-molecules can even be manipulated by laser tweezers with the optically trapped Au nanoparticles as handles. In this Letter, optical scattering torque arising from the coupled Au nanoparticles driven by circularly polarized light is theoretically presented. The coupled plasmon resonance modes boost the angular momentum transfer from photons to the Au nanoparticle dimers and trimers through light scattering, which does not bring any optical-heating side effect. The generated optical torques on the nanostructures highly depend on the plasmon coupling in the structures. The angular momentum transfer efficiencies from scattered photons to nanostructures can reach around 200\%. The results suggest that coupled plasmonic nanoparticle oligomers are promising candidates to construct optically driven rotary nanomotors that can be applied in biomedical applications.
Peer Review Status:Awaiting Review
Subjects: Optics >> Quantum optics submitted time 2023-02-19
Abstract： Tensor analytics lays mathematical basis for the prosperous promotion of multiway signal processing. To increase computing throughput, mainstream processors transform tensor convolutions to matrix multiplications to enhance parallelism of computing. However, such order-reducing transformation produces data duplicates and consumes additional memory. Here, we demonstrate an integrated photonic tensor flow processor without tensor-matrix transformation, which outputs the convolved tensor as the input tensor 'flows' through the processor. The hybrid manipulation of optical dimensions of wavelength, time, and space enables the direct representation and processing of high-order tensors in optical domain. In the proof-of-concept experiment, processing of multi-channel images and videos is accomplished at the frequency of 20 GHz. A convolutional neural network is demonstrated on the processor, which achieves an accuracy of 97.9 percent on action recognition.
Peer Review Status:Awaiting Review
Subjects: Optics >> Quantum optics submitted time 2023-02-19
Abstract： Missing second-order nonlinearity in centrosymmetric graphene overshadows its intriguing optical attribute. Here, we report redox-governed charge doping could effectively break the centrosymmetry of bilayer graphene (BLG), enabling a strong second harmonic generation (SHG) with a strength close to that of the well-known monolayer MoS2. Verified from control experiments with in situ electrical current annealing and electrically gate-controlled SHG, the required centrosymmetry breaking of the emerging SHG arises from the charge-doping on the bottom layer of BLG by the oxygen/water redox couple. Our results not only reveal that charge doping is an effective way to break the inversion symmetry of BLG despite its strong interlayer coupling but also indicate that SHG spectroscopy is a valid technique to probe molecular doping on two-dimensional materials.
Peer Review Status:Awaiting Review
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