分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: Optical metasurfaces with high-Q chiral resonances can boost light-matter interaction for various applications of chiral response for ultrathin, active, and nonlinear metadevices. Usually, such metasurfaces require sophisticated depth-resolved nanofabrication to realize subwavelength stereo-nanostructures, posing overwhelming challenges, especially in the short-wavelength range. Here, we suggest a novel planar design for chiral metasurfaces supporting bound states in the continuum (BICs) and demonstrate experimentally chiroptical responses with record-high Q-factors (Q=390) and near-perfect circular dichroism (CD=0.93) at optical frequencies. The symmetry-reduced meta-atoms are highly birefringent and support winding elliptical eigen-polarizations with opposite helicity surrounding the BIC polarization singularity, providing a convenient way for achieving maximal planar chirality tuned by either breaking in-plane symmetry or changing illumination direction. Such sharply resonant chirality realized in planar metasurfaces promises various practical applications in classical and quantum optics including chiral sensing, enantiomer selection, and chiral quantum emitters.
分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: Polaritons in polar biaxial crystals with extreme anisotropy offer a promising route to manipulate nanoscale light-matter interactions. The dynamical modulation of their dispersion is great significance for future integrated nano-optics but remains challenging. Here, we report a momentum-directed strategy, a coupling between the modes with extra momentum supported by the interface and in-plane hyperbolic polaritons, to tailor topological transitions of anisotropic polaritons in biaxial crystals. We experimentally demonstrate such tailored polaritons at the interface of heterostructures between graphene and {\alpha}-phase molybdenum trioxide ({\alpha}-MoO3). The interlayer coupling can be electrically modulated by changing the Fermi level in graphene, enabling a dynamic topological transition. More interestingly, we found that the topological transition occurs at a constant Fermi level when tuning the thickness of {\alpha}-MoO3. The momentum-directed strategy implemented by interface engineering offers new insights for optical topological transitions, which may shed new light for programmable polaritonics, energy transfer and neuromorphic photonics.