• Solid-like high harmonic generation from rotationally periodic systems

    分类: 光学 >> 量子光学 提交时间: 2023-02-19

    摘要: High harmonic generation (HHG) from crystals in strong laser fields has been understood by the band theory of solid, which is based on the periodic boundary condition (PBC) of translational invariant. For systems having PBC of rotational invariant, in principles an analogous Bloch theorem can be developed and applied. Taking a ring-type cluster of cyclo[18]carbon as a representative, we theoretically suggest a quasi-band model and study its HHG by solving time-dependent Liouville-von Neumann equation. Under the irradiation of circularly polarized laser, explicit selection rules for left-handed and right-handed harmonics are observed, while in linearly polarized laser field, cyclo[18]carbon exhibits solid-like HHG originated from intra-band oscillations and inter-band transitions, which in turn is promising to optically detect the symmetry and geometry of controversial structures. In a sense, this work presents a connection linking the high harmonics of gases and solids.

  • Generation of extreme ultraviolet laser by single-photon process

    分类: 光学 >> 量子光学 提交时间: 2023-02-19

    摘要: To generate laser with short wavelength is a bottle-neck problem in laser technology. The extreme ultraviolet (EUV) lasers are usually produced with low efficiency by nonlinear multi-photon process. Here we show the generation of 58.4 nm laser by a single-photon-excitation related stimulated anti-Stokes Raman scattering (ASRS) with an efficiency higher than that of high harmonic generation (HHG). Utilizing microwave excited helium in the metastable 1s2s state irradiated by a resonant femto-second 2058 nm laser, we obtain pulsed 58.4 nm laser with a divergence of 1.9 mrad, suggesting its coherent character. The pulse decay time of 426 ps shorter than the lifetime of spontaneous emission also shows its stimulated property. Our results show an applicable path towards up-conversion by single-photon process to generate intense laser with wavelength shorter than 58.4 nm.

  • Lens-free Optical Detection of Thermal Motion of a Sub-millimeter Sphere Diamagnetically Levitated in High Vacuum

    分类: 光学 >> 量子光学 提交时间: 2023-02-19

    摘要: Levitated oscillators with millimeter or sub-millimeter size are particularly attractive due to their potential role in studying various fundamental problems and practical applications. One of the crucial issues towards these goals is to achieve efficient measurements of oscillator motion, while this remains a challenge. Here we theoretically propose a lens-free optical detection scheme, which can be used to detect the motion of a millimeter or sub-millimeter levitated oscillator with a measurement efficiency close to the standard quantum limit with a modest optical power. We demonstrate experimentally this scheme on a 0.5 mm diameter micro-sphere that is diamagnetically levitated under high vacuum and room temperature, and the thermal motion is detected with high precision. Based on this system, an estimated acceleration sensitivity of $9.7 \times 10^{-10}\rm g/\sqrt{Hz}$ is achieved, which is more than one order improvement over the best value reported by the levitated mechanical system. Due to the stability of the system, the minimum resolved acceleration of $3.5\times 10^{-12}\rm g$ is reached with measurement times of $10^5$ s. This result is expected to have potential applications in the study of exotic interactions in the millimeter or sub-millimeter range and the realization of compact gravimeter and accelerometer.

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