Subjects: Optics >> Quantum optics submitted time 2023-02-19
Abstract: Autocorrelation measurement based on second-harmonic generation (SHG), the best-known technique for measuring the temporal duration of ultrashort pulses, could date back to the birth of ultrafast lasers. Here, we propose and experimentally demonstrate that such well-established technique can also be used to measure the orbital angular momentum of ultrashort Laguerre-Gauss (LG) pulses. By analysing the far-field pattern of the SHG signal, the full spatial structure of ultrashort LG pulses, including both azimuthal and radial indices, are unambiguously determined. Our results provide an important advancement for the well-established autocorrelation technique by extending it to reach its full potential in laser characterization, especially for structured ultrashort pulses.
Peer Review Status:Awaiting Review
Subjects: Optics >> Quantum optics submitted time 2023-02-19
Abstract: Orbital angular momentum (OAM) conservation plays an important role in shaping and controlling structured light with nonlinear optics. The OAM of a beam originating from three-wave mixing should be the sum or difference of the other two inputs because no light-matter OAM exchange occurs in parametric nonlinear interactions. Here, we report anomalous OAM conservation during parametric upconversion, in which a Hermite-Gauss mode signal interacts with a specially engineered pump capable of astigmatic transformation in a crystal, resulting in Laguerre-Gaussian mode sum-frequency generation (SFG). The anomaly here refers to the fact that the pump and signal carry no net OAM, while their SFG does. We show that the lost OAM with the opposite sign that maintains OAM conservation in the system is hidden in the residual pump. This unexpected OAM selection rule improves our understanding of OAM conservation in parametric nonlinear systems and may inspire new ideas for controlling OAM states via nonlinear optics, especially in quantum applications.
Peer Review Status:Awaiting Review
Subjects: Optics >> Quantum optics submitted time 2023-02-19
Abstract: Vectorial structured light with spatially varying amplitude, phase, and polarization is reshaping many areas of modern optics, including nonlinear optics, as diverse parametric processes can be used to explore interactions between such complex vector fields, extending the frontiers of optics to new physical phenomena. However, the most basic nonlinear application, i.e., frequency conversion, still remains challenging for vectorial structured light since parametric processes are polarization dependent, leading to a change in the spatial topological structure of signals. In this work, to break this fundamental limit, we propose a novel conformal frequency conversion scheme that allows to maintain the full spatial structure of vectorial structured light in the conversion; and systematically examine its spatial polarization independence based on non-degenerate sum-frequency generation with type-0 phase matching. This proof-of-principle demonstration paves the way for a wide range of applications requiring conformal frequency conversion, and, particularly, to implement frequency interfaces with multimodal communication channels, high-dimensional quantum states, and polarization-resolved upconversion imaging.
Peer Review Status:Awaiting Review