分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: The interaction of magnetic dipole (MD) emitters and common photonic cavities is usually weak, which is partially due to the low magnetic near field enhancements of the cavities. Here, we show that whispering gallery modes (WGMs) of a subwavelength dielectric cavity can not only greatly boost the emission rate of a MD emitter but also bring efficient couplings between coherent MD emitters. In a WGM cavity, the maximal emission rate ({\gamma}max) of a single emitter occurs at an antinode of the field pattern. The emission of the MD emitter can also be greatly affected by another coherent one depending on the magnetic field response of the WGM. The maximal contribution can also reach {\gamma}max. Notably, the cooperative emission rate of the coherent MD emitters does not decay with distance in the considered range due to the high-quality feature of a WGM. In contrast to the emission, the absorption of an emitter is hardly affected by the coherent couplings between emitters mediated by a WGM. The difference between the performances of emission and absorption is highly related to the excitation behaviors of WGMs. Our results are important for enhanced magnetic light-matter interactions.
分类: 光学 >> 量子光学 提交时间: 2023-02-19
摘要: Utilization of triplet excitons, which generally emit poorly, is always fundamental to realize highly efficient organic light-emitting diodes (LEDs). While triplet harvest and energy transfer via electron exchange between triplet donor and acceptor are fully understood in doped organic phosphorescence and delayed fluorescence systems, the utilization and energy transfer of triplet excitons in quasi-two-dimensional (quasi-2D) perovskite are still ambiguous. Here, we use an orange-phosphorescence-emitting ultrathin organic layer to probe triplet behavior in the sky-blue-emitting quasi-2D perovskite. The delicate white LEDs architecture enables a carefully tailored Dexter-like energy-transfer mode that largely rescues the triplet excitons in quasi-2D perovskite. Our white organic-inorganic LEDs achieve maximum forward-viewing external quantum efficiency of 8.6% and luminance over 15000 cd m-2, exhibiting a significant efficiency enhancement versus the corresponding sky-blue perovskite LED (4.6%). The efficient management of energy transfer between excitons in quasi-2D perovskite and Frenkel excitons in organic layer opens the door to fully utilizing excitons for white organic-inorganic LEDs.