Subjects: Optics >> Quantum optics submitted time 2023-02-19
Jinyu Pan
Yifei Chen
Zhiyuan Huang
Cheng Zhang
Tiandao Chen
Donghan Liu
Ding Wang
Meng Pang
Yuxin Leng
Abstract： Femtosecond light pulses carrying optical angular momentums (OAMs), possessing intriguing properties of helical phase fronts and ultrafast temporal profiles, enable many applications in nonlinear optics, strong-field physics and laser micro-machining. While generation of OAM-carrying ultrafast pulses and their interactions with matters have been intensively studied in experiments, three-dimensional characterization of ultrafast OAM-carrying light beams in spatio-temporal domain has, however, proved difficult to achieve. Conventional measurement schemes rely on the use of a reference pulsed light beam which needs to be well-characterized in its phase front and to have sufficient overlap and coherence with the beam under test, largely limiting practical applications of these schemes. Here we demonstrate a self-referencing set-up based on a tilted interferometer that can be used to measure complete spatio-temporal information of OAM-carrying femtosecond pulses with different topological charges. Through scanning one interferometer arm, the spectral phase over the pulse spatial profile can be obtained using the tilted interference signal, and the temporal envelope of the light field at one particular position around its phase singularity can be retrieved simultaneously, enabling three-dimensional beam reconstruction. This self-referencing technique, capable of measuring spatio-temporal ultrafast optical-vortex beams, may find many applications in fields of nonlinear optics and light-matter interactions.
Peer Review Status:
Awaiting Review
Subjects: Optics >> Quantum optics submitted time 2023-02-19
Abstract： Dirac Fermion, which is the low energy collective excitation near the Dirac cone in monolayer graphene, have gained great attention by low energy Terahertz probe. In the case of undoped graphene, it has been generally understood that the ultrafast terahertz thermal relaxation is mostly driven by the electron-phonon coupling (EOP), which can be prolonged to tens and hundreds of picoseconds. However, for the high doped graphene, which manifests the negative photoinduced terahertz conductivity, there is still no consensus on the dominant aspects of the cooling process on a time scale of a few picoseconds. Here, the competition between the disorders assisted defect scattering and the electron-phonon coupling process in the cooling process of the graphene terahertz dynamics is systematically studied and disentangled. We verify experimentally that the ultrafast disorder assisted lattice-phonon interaction, rather than the electron-phonon coupling process, would play the key role in the ultrafast thermal relaxation of the terahertz dynamics. Furthermore, the cooling process features robustness which is independent on the pump wavelength and external temperature. Our finding is expected to propose a considerable possible cooling channel in CVD-graphene and to increase the hot electron extracting efficiency for the design of graphene-based photoconversion devices.
Peer Review Status:Awaiting Review
Subjects: Optics >> Quantum optics submitted time 2023-02-19
Chuanchuan Yan
Hongyang Li
Zhiyuan Huang
Xinliang Wang
Donghan Liu
Xingyan Liu
Jinyu Pan
Zhuozhao Luo
Fei Yang
Yu Zheng
Ruochen Yin
Haihu Yu
Yuxin Leng
Liwei Song
Meng Pang
Xin Jiang
Abstract： We demonstrate the stable and flexible light delivery of multi-{\mu}J, sub-200-fs pulses over a ~10-m-long vacuumized anti-resonant hollow-core fiber (AR-HCF), which was successfully used for high-performance pulse synchronization. Compared with the pulse train launched into the AR-HCF, the transmitted pulse train out of the fiber exhibits excellent stabilities in pulse power and spectrum, with pointing stability largely improved. The walk-off between the fiber-delivery and the other free-space-propagation pulse trains, in an open loop, was measured to be <6 fs root-mean-square (RMS) over 90 minutes, corresponding to a relative optical-path variation of <2x10-7. This walk-off can be further suppressed to ~2 fs RMS simply using an active control loop, highlighting the great application potentials of this AR-HCF set-up in large-scale laser and accelerator facilities.
Peer Review Status:Awaiting Review
Subjects: Optics >> Quantum optics submitted time 2023-02-19
Yuqing Zou
Qiu-Shi Ma
Zeyu Zhang
Ruihua Pu
Wenjie Zhang
Peng Suo
Jiaming Chen
Di Li
Hong Ma
Xian Lin
Yuxin Leng
Weimin Liu
Juan Du
Guohong Ma
Abstract： In this study,we combined time-resolved terahertz spectroscopy along with transient absorption spectroscopy to revisit the interlayer non-equilibrium carrier dynamics in largely lateral size Gr/MoS2 heterostructure fabricated with chemical vapor deposition method. Our experimental results reveal that, with photon-energy below the A-exciton of MoS2 monolayer, hot electrons transfer from graphene to MoS2 takes place in time scale of less than 0.5 ps, resulting in ultrafast formation of interfacial exciton in the heterostructure, subsequently, recombination relaxation of the interfacial exciton occurs in time scale of ~18 ps. A new model considering carrier heating and photogating effect in graphene is proposed to estimate the amount of carrier transfer in the heterostructure, which shows a good agreement with experimental result. Moreover, when the photon-energy is on-resonance with the A-exciton of MoS2, photogenerated holes in MoS2 are transferred to graphene layer within 0.5 ps, leading to the formation of interfacial exciton, the subsequent photoconductivity (PC) relaxation of graphene and bleaching recovery of A-exciton in MoS2 take place around ~10 ps time scale, ascribing to the interfacial exciton recombination. The faster recombination time of interfacial exciton with on-resonance excitation could come from the reduced interface barrier caused by bandgap renormalization effect. Our study provides deep insight into the understanding of interfacial charge transfer as well as the relaxation dynamics in graphene-based heterostructures, which are promising for the applications of graphene-based optoelectronic devices.
Peer Review Status:Awaiting Review
Subjects: Optics >> Quantum optics submitted time 2023-02-19
Cheng Zhang
Tiandao Chen
Jinyu Pan
Zhiyuan Huang
Donghan Liu
Ding Wang
Fei Yu
Dakun Wu
Yu Zheng
Ruochen Yin
Xin Jiang
Meng Pang
Yuxin Leng
Ruxin Li
Abstract： High-energy ultraviolet pulse generation in gas-filled hollow capillary fibers (HCFs) through dispersive-wave-emission process, has attracted considerable attentions in recent several years due to its great application potentials in ultraviolet spectroscopy and photochemistry. While the ability of this technique to deliver high-energy, ultrafast ultraviolet pulses is widely recognized, few-fs duration of {\mu}J-level dispersive-wave (DW) pulses has, however, escaped direct measurements. In this letter, we demonstrate that using several chirped mirrors, few-fs ultraviolet DW pulses can be obtained in atmosphere environment without the use of vacuum chambers. The pulse temporal profiles, measured using a self-diffraction frequency-resolved optical gating set-up, exhibit full-width-half-maximum pulse widths of 9.6 fs at 384 nm and 9.4 fs at 430 nm, close to the Fourier-transform limits. Moreover, theoretical and experimental studies reveal the strong influences of driving pulse energy and HCF length on temporal width and shape of the measured DW pulses. The ultraviolet pulses obtained in atmosphere environment with {\mu}J-level pulse energy, few-fs pulse width and broadband wavelength tunability are ready to be used in many applications.
Peer Review Status:Awaiting Review
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