Subjects: Optics >> Quantum optics submitted time 2023-02-19
Abstract： High harmonic generation (HHG) from crystals in strong laser fields has been understood by the band theory of solid, which is based on the periodic boundary condition (PBC) of translational invariant. For systems having PBC of rotational invariant, in principles an analogous Bloch theorem can be developed and applied. Taking a ring-type cluster of cyclo[18]carbon as a representative, we theoretically suggest a quasi-band model and study its HHG by solving time-dependent Liouville-von Neumann equation. Under the irradiation of circularly polarized laser, explicit selection rules for left-handed and right-handed harmonics are observed, while in linearly polarized laser field, cyclo[18]carbon exhibits solid-like HHG originated from intra-band oscillations and inter-band transitions, which in turn is promising to optically detect the symmetry and geometry of controversial structures. In a sense, this work presents a connection linking the high harmonics of gases and solids.
Peer Review Status:
Awaiting Review
Subjects: Optics >> Quantum optics submitted time 2023-02-19
Abstract： As a promising avenue to obtain new extreme ultraviolet light source and detect electronic properties, high-harmonic generation (HHG) has been actively developed in both theory and experiment. In solids lacking inversion symmetry, when electrons undergo a nonadiabatic transition, a directional charge shift occurs and is characterized by shift vector, which measures the real-space shift of the photoexcited electron and hole. For the first time, we have revealed that shift vector plays prominent roles in the real-space tunneling mechanism of three-step model for electrons under strong laser fields. Since shift vector is determined by the topological properties of related wave functions, we expect HHG with its contribution can provide direct knowledge on the band topology in noncentrosymmetric topological insulators (TIs). In both Kane-Mele model and realistic material BiTeI, we have found that the shift vector reverses when band inversion happens during the topological phase transition between normal and topological insulators. Under oscillating strong laser fields, the reversal of shift vector leads to completely opposite radiation time of high-order harmonics. This makes HHG a feasible all-optical strong-field method to directly identify the band inversion in non-centrosymmetric TIs.
Peer Review Status:Awaiting Review
Subjects: Optics >> Quantum optics submitted time 2023-02-19
Abstract： Ultraviolet single-photon detector (UVSPD) provides a key tool for the applications requiring ultraweak light detection in the wavelength band. Here, we report a 4H-SiC single-photon avalanche diode (SPAD) based free-running UVSPD with ultralow afterpulse probability. We design and fabricate the 4H-SiC SPAD with a beveled mesa structure, which exhibits the characteristic of ultralow dark current. We further develop a readout circuit of passive quenching and active reset with tunable hold-off time setting to considerably suppress the afterpulsing effect. The nonuniformity of photon detection efficiency (PDE) across the SPAD active area with a diameter of $\sim$ 180 $\mu$m is investigated for performance optimization. The compact UVSPD is then characterized, exhibiting a typical performance of 10.3% PDE, 133 kcps dark count rate and 0.3% afterpulse probability at 266 nm. Such performance indicates that the compact UVSPD could be used for practical ultraviolet photon-counting applications
Peer Review Status:Awaiting Review
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